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Weak base-promoted selective rearrangement of oxaziridines to amides via visible-light photoredox catalysis

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Abstract
The selective rearrangement of oxaziridines to amides via a single electron transfer (SET) pathway is unexplored. In this study, we present a weak base-promoted selective rearrangement of oxaziridines to amides via visible-light photoredox catalysis. The developed method shows excellent functional group tolerance with a broad substrate scope and good to excellent yields. Furthermore, control experiments and density functional theory (DFT) calculations are performed to gain insight into the reactivity and selectivity.
Author(s)
김란희박세훈박진우상국장광석정재훈
Issued Date
2021
Type
Article
DOI
10.1039/D1CC03855A
URI
https://oak.ulsan.ac.kr/handle/2021.oak/9655
https://ulsan-primo.hosted.exlibrisgroup.com/primo-explore/fulldisplay?docid=TN_cdi_proquest_miscellaneous_2569619843&context=PC&vid=ULSAN&lang=ko_KR&search_scope=default_scope&adaptor=primo_central_multiple_fe&tab=default_tab&query=any,contains,Weak%20base-promoted%20selective%20rearrangement%20of%20oxaziridines%20to%20amides%20via%20visible-light%20photoredox%20catalysis&offset=0&pcAvailability=true
Publisher
CHEMICAL COMMUNICATIONS
Location
영국
Language
영어
ISSN
1359-7345
Citation Volume
57
Citation Number
78
Citation Start Page
9995
Citation End Page
9998
Appears in Collections:
Natural Science > Chemistry
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